You can display the number of items by using the DataItem.Items.Count path, note that we expose the items collection, and we use this in the tooltip to display the detail of all the elements grouped in the Other bucket.
<TextBlock Text="{Binding Path=DataItem.Items.Count}"/>
To show the accumulated value or percentage you can use ToolTipConverter, the advantage of using this is that it knows about Axis settings, e.g. if you set the Axis.Format to currency it will show the currency sign when displaying the value, e.g.
xmlns:cfxConverters="clr-namespace:ChartFX.WPF.Converters;assembly=ChartFX.WPF"
<DataTemplate.Resources>
<cfxConverters:TooltipConverter x:Key="MyTooltipConverter"/>
</DataTemplate.Resources>
<TextBlock>
<TextBlock.Text>
<Binding Path="Self" Converter="{StaticResource MyTooltipConverter}" ConverterParameter="V: %v P: %p%%" />
</TextBlock.Text>
</TextBlock>
JuanC